2-Fluoro-3-nitrobenzoic acid

CAS Number 317-46-4
Molecular Formula C₇H₄FNO₄
Molecular Weight 185.11 g/mol
Purity ≥99.5%
Appearance Light-yellow crystalline solid

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Product Description

2-Fluoro-3-nitrobenzoic acid is an exceptionally versatile building block for installing fluorinated, nitro-aromatic or benzoic-acid motifs into more complex targets. Prepared on scale by low-temperature nitration of 2-fluorobenzoic acid, it is soluble in hot water and common polar organic solvents and is traded commercially as a high-purity intermediate. Its reactivity profile is exploited across three main sectors: in medicinal chemistry it is a key precursor to kinase inhibitors and other fluorinated targeted therapeutics; in crop science it is converted into specialty benzoic-acid herbicides and insecticides; and in materials research it serves as a fluorinated monomer or linker for liquid-crystalline and high-performance polymeric systems.

Synthesis and Production

Main Synthesis Routes:

  1. Chromic Acid Oxidation (Industrial Scale)

    • Starting Material: 2-Fluoro-3-nitrotoluene

    • Conditions: Acetic acid solvent, concentrated H₂SO₄, dropwise addition of CrO₃ in water at 95 °C, maintained for 3 hours.

    • Yield: 62–65%.

  2. Salicylic Acid Multi-Step Derivatization

    • Salicylic acid → Esterification → Nitration → Chlorination → Chloro-fluoro exchange → Hydrolysis.

    • Suitable for large-scale production; lower cost and easier separation of intermediates.

  3. Nitration Method

    • Nitration of 2-fluorobenzoic acid using mixed acid (HNO₃/H₂SO₄).

    • Temperature control (0–10 °C) required to avoid over-nitration.

Production Notes: An industrially relevant fluorinated aromatic acid used as a fine chemical intermediate in both laboratory and industrial settings.

Uses and Applications

  1. Pharmaceutical Intermediate

    • Key building block for fluorinated targeted drugs (e.g., kinase inhibitors such as Dabrafenib).

    • Starting material for quinolone and benzimidazole antibacterial/antiviral agents.

    • Used in constructing fluorinated bioactive molecules.

  2. Agrochemical Intermediate

    • Synthesis of fluorinated benzoic acid-based herbicides, fungicides, and insecticides.

    • Can be reduced and rearranged to prepare fluorinated aniline pesticides.

  3. Materials and Dyes

    • Precursor for fluorinated liquid crystal monomers and polymer materials.

    • Used in fluorescent dye synthesis (nitro group reducible to amino for coupling).

  4. Research Building Block

    • Aromatic module for Suzuki, Buchwald, nucleophilic substitution, and other coupling reactions.

    • Valuable for structure–activity relationship (SAR) optimization.

Chemical and Physical Properties

Property Description
Molecular Formula C₇H₄FNO₄
Molecular Weight 185.11 g/mol
CAS No. 317-46-4 (also listed: 4715-07-3, 401-96-7)
Appearance Pale yellow to off-white crystalline powder
Melting Point ~138–160 °C (literature varies, commonly 145–160 °C)
Boiling Point ~347.6 °C (predicted)
Solubility Slightly soluble in water; soluble in ethanol, methanol, ethyl acetate, DMF, DMSO
Acidity (pKa) ~2.32–4.2 (stronger acid due to electron-withdrawing fluoro and nitro groups)
LogP 1.3–1.43 (moderate lipophilicity)
Hydrogen Bond Donor/Acceptor 1 / 5
Polar Surface Area ~83.1 Ų
Chemical Stability Slowly decarboxylates if heated above 180 °C; avoid prolonged melting.

Key Chemical Features:

  • Ortho-fluoro and meta-nitro groups are strong electron-withdrawing substituents, enhancing electrophilicity.

  • Nitro group can be reduced to an amine (e.g., using SnCl₂/HCl or Pd/C-H₂).

  • Fluorine atom can undergo nucleophilic substitution under forcing conditions (e.g., with NaOH or amines).

Safety and Handling

GHS Hazard Classification:

  • Pictogram: ⚠️ (Irritant)

  • Signal Word: Warning

  • Hazard Statements:

    • H315: Causes skin irritation

    • H319: Causes serious eye irritation

    • H335: May cause respiratory irritation

Precautionary Measures:

  • Use personal protective equipment: gloves, safety goggles, dust mask.

  • Handle in a well-ventilated area to avoid dust inhalation.

  • Avoid contact with strong oxidizers, reducing agents, and bases.

Storage:

  • Store in a tightly sealed container in a cool, dry place (recommended 2–8 °C).

  • Keep away from heat, sparks, and light.

  • Store separately from metal powders and incompatible materials.

Environmental & Toxicity:

  • Toxic to aquatic life.

  • Prevent release into the environment.

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